Specific heat measurements in magnetic fields have been performed on !-Dy2S3 single crystal that shows successive magnetic transitions at TN1 = 11.4 K and TN2 = 6.4 K. The specific heat in no magnetic field exhibits sharp peaks at both temperatures of TN1 and TN2.The change of magnetic entropy across each transition is estimated as Rln2/2 per mol-Dy,which suggests magnetic moments on only one Dy site between two crystallographically inequivalent Dy sites order at each transition temperature. When the magnetic field is applied along the b-axis of the orthorhombic system, two peaks of the specific heat shift toward lower temperatures. On the other hand, the magnetic field perpendicular to the b-axis shifts the peaks toward higher temperatures. The TN1 shifts to 9.6 K (H// b) and 12.5 K (H⊥b) under the magnetic field of 2 T. The peak of TN2 broadens gradually with increasing magnetic field for each direction, and the peak is consequently obscure under the field of 2 T.
Specific-heat study on successive magnetic transitions in α-Dy2S3 single crystals under magnetic fields
JKPS_63_3_571_574
(977.79KB)
