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Electronic structure of Cu1-xNixRh2S4 and CuRh2Se4 : Band-structure calculations, X-ray photoemission, and fluorescence measurements
http://hdl.handle.net/10258/250
http://hdl.handle.net/10258/2507a5f9279-b9e9-4659-8c26-7cf0a35f7e4c
名前 / ファイル | ライセンス | アクション |
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PR-B_61_4230.pdf (155.6 kB)
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Item type | 学術雑誌論文 / Journal Article.(1) | |||||
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公開日 | 2007-09-26 | |||||
タイトル | ||||||
言語 | en | |||||
タイトル | Electronic structure of Cu1-xNixRh2S4 and CuRh2Se4 : Band-structure calculations, X-ray photoemission, and fluorescence measurements | |||||
言語 | ||||||
言語 | eng | |||||
キーワード | ||||||
言語 | en | |||||
主題Scheme | Other | |||||
主題 | band structure | |||||
キーワード | ||||||
言語 | en | |||||
主題Scheme | Other | |||||
主題 | copper compounds | |||||
キーワード | ||||||
言語 | en | |||||
主題Scheme | Other | |||||
主題 | electronic density of states | |||||
キーワード | ||||||
言語 | en | |||||
主題Scheme | Other | |||||
主題 | fluorescence | |||||
キーワード | ||||||
言語 | en | |||||
主題Scheme | Other | |||||
主題 | nickel compounds | |||||
キーワード | ||||||
言語 | en | |||||
主題Scheme | Other | |||||
主題 | rhodium compounds | |||||
キーワード | ||||||
言語 | en | |||||
主題Scheme | Other | |||||
主題 | superconducting transition | |||||
キーワード | ||||||
言語 | en | |||||
主題Scheme | Other | |||||
主題 | temperature | |||||
キーワード | ||||||
言語 | en | |||||
主題Scheme | Other | |||||
主題 | X-ray emission spectra | |||||
キーワード | ||||||
言語 | en | |||||
主題Scheme | Other | |||||
主題 | X-ray photoelectron spectra | |||||
資源タイプ | ||||||
資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
資源タイプ | journal article | |||||
アクセス権 | ||||||
アクセス権 | open access | |||||
アクセス権URI | http://purl.org/coar/access_right/c_abf2 | |||||
著者 |
HART, G.L.W.
× HART, G.L.W.× PICKETT, W.E.× KURMAEV, E. Z.× HARTMANN, D.× NEUMANN, M.× MOEWES, A.× EDERER, D. L.× ENDO, R.× TANIGUCHI, K.× 永田, 正一 |
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抄録 | ||||||
内容記述タイプ | Abstract | |||||
内容記述 | The electronic structure of spinel-type Cu1-xNixRh2S4 (x=0.0, 0.1, 0.3, 0.5, 1.0) and CuRh2Se4 compounds has been studied by means of X-ray photoelectron (XPS) and fluorescent spectroscopy. Cu L3, Ni L3, S L2,3, and Se M2,3 X-ray emission spectra (XES) were measured near thresholds at Beamline 8.0 of the Lawrence Berkeley Laboratory's Advanced Light Source. XES measurements of the constituent atoms of these compounds, reduced to the same binding energy scale, are found to be in excellent agreement with XPS valence bands. The calculated XES spectra which include dipole matrix elements show that the partial density of states reproduce experimental spectra quite well. States near the Fermi level (EF) have strong Rh d and S(Se) p character in all compounds. In NiRh2S4 the Ni 3d states contribute strongly at EF, whereas in both Cu compounds the Cu 3d bands are only ~1 eV wide and centered ~2.5 eV below EF, leaving very little 3d character at EF. The density of states at the Fermi level is less in NiRh2S4 than in CuRh2S4. This difference may contribute to the observed decrease, as a function of Ni concentration, in the superconducting transition temperature in Cu1-xNixRh2S4. The density of states of the ordered alloy Cu0.5Ni0.5Rh2S4 shows behavior that is more “split-band”-like than “rigid-band”-like. | |||||
言語 | en | |||||
書誌情報 |
en : Physical review. Third series. B, Condensed matter and materials physics 巻 61, 号 6, p. 4230-4237, 発行日 2000-02-01 |
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出版者 | ||||||
言語 | en | |||||
出版者 | The American Physical Society | |||||
出版者版へのリンク | ||||||
10.1103/PhysRevB.61.4230 | ||||||
https://doi.org/10.1103/PhysRevB.61.4230 | ||||||
DOI | ||||||
関連タイプ | isIdenticalTo | |||||
識別子タイプ | DOI | |||||
関連識別子 | 10.1103/PhysRevB.61.4230 | |||||
論文ID(NAID) | ||||||
関連タイプ | isIdenticalTo | |||||
識別子タイプ | NAID | |||||
関連識別子 | 120000802040 | |||||
日本十進分類法 | ||||||
主題Scheme | NDC | |||||
主題 | 428.4 | |||||
ISSN | ||||||
収録物識別子タイプ | PISSN | |||||
収録物識別子 | 10980121 | |||||
書誌レコードID | ||||||
収録物識別子タイプ | NCID | |||||
収録物識別子 | AA11187113 | |||||
権利 | ||||||
言語 | en | |||||
権利情報 | © 2000 The American Physical Society | |||||
著者版フラグ | ||||||
出版タイプ | VoR | |||||
出版タイプResource | http://purl.org/coar/version/c_970fb48d4fbd8a85 | |||||
フォーマット | ||||||
内容記述タイプ | Other | |||||
内容記述 | application/pdf |